Longitudinal spin relaxation in simple stochastic models for disordered systems

verfasst von: P. Borgs, K. W. Kehr, P. Heitjans
Abstract: The relaxation of single probe spins was investigated for simple models of systems with quenched disorder. The spin relaxation was calculated for a two-site model with arbitrarily oriented magnetic fields and the result was averaged over various distributions of the fields, and of the hopping rates of the spin. On an intermediate time scale, a modified Kubo-Toyabe behavior is obtained for large hopping rates, in agreement with recent SR experiments. A stretched-exponential decay of the spin polarization is obtained at longer times. The Kohlrausch exponent is found to be field and hopping-rate dependent, in qualitative agreement with recent NMR and -NMR experiments. The resulting longitudinal relaxation rate still does not show the significant deviations from the Bloembergen-Purcell-Pound (BPP) behavior that are typical for glassy systems. Therefore, the random two-frequency model was extended to include time-dependent renewals of the environment. This modification may yield asymmetric peaks for the longitudinal relaxation rate in the BPP plot for very large renewal rates.
Organisationseinheit(en): Institut für Physikalische Chemie und Elektrochemie
Externe Organisation(en): Forschungszentrum Jülich
Typ: Artikel
Journal: Physical Review B
Band: 52
Seiten: 6668-6683
Anzahl der Seiten: 16
ISSN: 0163-1829
Publikationsdatum: 1995
Publikationsstatus: Veröffentlicht
Peer-reviewed: Ja
ASJC Scopus Sachgebiete: Physik der kondensierten Materie
Elektronische Version(en): https://doi.org/10.1103/PhysRevB.52.6668 (Zugang: Unbekannt)

BibTeX

@article{a9320f98efba4ef0a08b6588c358dcbb,
title = "Longitudinal spin relaxation in simple stochastic models for disordered systems",
abstract = "The relaxation of single probe spins was investigated for simple models of systems with quenched disorder. The spin relaxation was calculated for a two-site model with arbitrarily oriented magnetic fields and the result was averaged over various distributions of the fields, and of the hopping rates of the spin. On an intermediate time scale, a modified Kubo-Toyabe behavior is obtained for large hopping rates, in agreement with recent SR experiments. A stretched-exponential decay of the spin polarization is obtained at longer times. The Kohlrausch exponent is found to be field and hopping-rate dependent, in qualitative agreement with recent NMR and -NMR experiments. The resulting longitudinal relaxation rate still does not show the significant deviations from the Bloembergen-Purcell-Pound (BPP) behavior that are typical for glassy systems. Therefore, the random two-frequency model was extended to include time-dependent renewals of the environment. This modification may yield asymmetric peaks for the longitudinal relaxation rate in the BPP plot for very large renewal rates.",
author = "P. Borgs and Kehr, {K. W.} and P. Heitjans",
year = "1995",
doi = "10.1103/PhysRevB.52.6668",
language = "English",
volume = "52",
pages = "6668--6683",
journal = "Physical Review B",
issn = "0163-1829",
publisher = "American Institute of Physics",
number = "9",
}